Failed to evaluate Schwarz integrals 2

Dear QChem community,

I am having problems using the ANO-RCC-TZVP basis set with NBr molecule taken from https://www.basissetexchange.org/, since there are no ANO basis sets available directly in its standard basis set library. I have used it in a simple HF calculation:

$molecule
0 3
N1
Br2 N1 ss
ss = 1.787
$end

$rem
METHOD 		   HF
BASIS              GEN
PURECART 111
UNRESTRICTED       FALSE
MEM_TOTAL          120000
MEM_STATIC         10000
$end

$basis
N     0
S   14   1.00
  74761.715                  0.00011826
  11123.654                  0.00051729
   2512.6857                 0.00226666
    703.77729                0.00914529
    225.47879                0.03239343
     79.615810               0.09770793
     30.237283               0.23170368
     12.263622               0.37688989
      5.2650860              0.31774207
      2.3334710              0.08211309
       .90185600             0.00331209
       .35833600             0.00372082
       .14109300             0.00316542
       .04938300             0.00045958
S   14   1.00
  74761.715                 -0.00071963
  11123.654                 -0.00253501
   2512.6857                -0.01619162
    703.77729               -0.03433297
    225.47879               -0.25361838
     79.615810              -0.15285691
     30.237283              -1.74822219
     12.263622               5.96579588
      5.2650860             -8.37442240
      2.3334710              6.88087642
       .90185600            -4.21773591
       .35833600             2.50135114
       .14109300            -1.17693319
       .04938300             0.32991955
S   14   1.00
  74761.715                 -0.00002707
  11123.654                 -0.00011837
   2512.6857                -0.00052038
    703.77729               -0.00210293
    225.47879               -0.00756820
     79.615810              -0.02346767
     30.237283              -0.06042901
     12.263622              -0.11705491
      5.2650860             -0.15553215
      2.3334710             -0.02468935
       .90185600             0.36250545
       .35833600             0.55508450
       .14109300             0.21483769
       .04938300             0.00898385
S   14   1.00
  74761.715                  0.00038509
  11123.654                  0.00170361
   2512.6857                 0.00724038
    703.77729                0.03017310
    225.47879                0.09828483
     79.615810               0.30235071
     30.237283               0.45939279
     12.263622               0.38497667
      5.2650860             -4.02509451
      2.3334710              6.08455283
       .90185600            -5.72112852
       .35833600             4.57890413
       .14109300            -2.77418964
       .04938300             0.99596354
S   14   1.00
  74761.715                  0.00001876
  11123.654                  0.00008118
   2512.6857                 0.00036590
    703.77729                0.00144304
    225.47879                0.00553184
     79.615810               0.01724359
     30.237283               0.05279548
     12.263622               0.11528813
      5.2650860              0.23525939
      2.3334710             -0.04896387
       .90185600            -1.02321774
       .35833600            -0.14815866
       .14109300             1.02155754
       .04938300             0.17240183
S   14   1.00
  74761.715                 -0.00004944
  11123.654                 -0.00020734
   2512.6857                -0.00098676
    703.77729               -0.00354228
    225.47879               -0.01480997
     79.615810              -0.03791568
     30.237283              -0.12570554
     12.263622              -0.14562395
      5.2650860             -0.47325710
      2.3334710              0.89687591
       .90185600             1.25975854
       .35833600            -2.53303820
       .14109300             0.89234315
       .04938300             0.54477257
S   14   1.00
  74761.715                  0.00007582
  11123.654                  0.00032043
   2512.6857                 0.00150488
    703.77729                0.00549511
    225.47879                0.02246954
     79.615810               0.05918803
     30.237283               0.18754539
     12.263622               0.20818024
      5.2650860              0.68908242
      2.3334710             -2.95142438
       .90185600             2.95584270
       .35833600            -0.63542189
       .14109300            -1.46054685
       .04938300             1.30730182
S   14   1.00
  74761.715                 -0.00019845
  11123.654                 -0.00092629
   2512.6857                -0.00355073
    703.77729               -0.01713801
    225.47879               -0.04629375
     79.615810              -0.18520613
     30.237283              -0.20645116
     12.263622              -0.60788741
      5.2650860              1.37705967
      2.3334710              0.54073010
       .90185600            -3.28568898
       .35833600             4.68302060
       .14109300            -3.92434152
       .04938300             1.70463830
P   9   1.00
    126.66657                0.00123363
     29.837389               0.00949341
      9.3940380              0.04293962
      3.4051040              0.13629254
      1.3500000              0.29213625
       .55769600             0.38878876
       .23244900             0.29468014
       .09426400             0.08012876
       .03299200             0.00054052
P   9   1.00
    126.66657                0.00265721
     29.837389               0.02785593
      9.3940380              0.10179588
      3.4051040              0.50382639
      1.3500000              0.51531948
       .55769600            -1.25011385
       .23244900             0.02506035
       .09426400             0.70769297
       .03299200             0.01393975
P   9   1.00
    126.66657               -0.00146623
     29.837389              -0.01182148
      9.3940380             -0.04983126
      3.4051040             -0.17309042
      1.3500000             -0.47323708
       .55769600            -0.20551132
       .23244900             0.59103798
       .09426400             0.45117968
       .03299200             0.01367472
P   9   1.00
    126.66657               -0.00480802
     29.837389              -0.04290371
      9.3940380             -0.24285598
      3.4051040             -0.96689679
      1.3500000              1.42757381
       .55769600            -0.01174627
       .23244900            -1.36761749
       .09426400             1.05460864
       .03299200             0.04493039
P   9   1.00
    126.66657                0.01143981
     29.837389               0.01738306
      9.3940380              0.63813118
      3.4051040              0.14922934
      1.3500000             -1.94346544
       .55769600             3.14534959
       .23244900            -2.80443021
       .09426400             1.20770873
       .03299200             0.11723832
P   9   1.00
    126.66657               -0.02724692
     29.837389              -0.01351039
      9.3940380             -1.36800321
      3.4051040              2.45337606
      1.3500000             -2.43539844
       .55769600             1.54058001
       .23244900            -0.24945376
       .09426400            -0.77957565
       .03299200             0.88417010
P   9   1.00
    126.66657                0.01148260
     29.837389               0.00502035
      9.3940380              0.88044987
      3.4051040             -1.84976099
      1.3500000              2.51799697
       .55769600            -2.92787924
       .23244900             3.05420923
       .09426400            -2.63360399
       .03299200             1.52744713
D   4   1.00
      2.7500000              0.14730165
       .96250000             0.55021826
       .33687500             0.44525604
       .11790600             0.04942869
D   4   1.00
      2.7500000             -0.44408434
       .96250000            -0.59138480
       .33687500             0.86513362
       .11790600             0.16640483
D   4   1.00
      2.7500000              1.13751946
       .96250000            -1.13805664
       .33687500             0.21203512
       .11790600             0.49902803
D   4   1.00
      2.7500000             -0.65117982
       .96250000             1.23159374
       .33687500            -1.57251290
       .11790600             1.28752711
F   3   1.00
      1.8000000              0.33209008
       .72000000             0.56991055
       .28800000             0.28683273
F   3   1.00
      1.8000000             -0.81770852
       .72000000             0.08144264
       .28800000             0.74971670
F   3   1.00
      1.8000000              1.06490976
       .72000000            -1.65849607
       .28800000             1.12632841
G   2   1.00
      0.9000000              0.93831502
      0.3600000              0.10169702
G   2   1.00
      0.9000000             -0.77885866
      0.3600000              1.21520106
****
Br     0
S   20   1.00
17028964.9                  -0.00013462
2186438.81                  -0.00044229
 426256.871                 -0.00130094
 105103.670                 -0.00350261
  30487.8213                -0.00918340
   9970.05197               -0.02405403
   3574.64352               -0.06239651
   1376.85529               -0.15033393
    560.732930              -0.29659185
    238.734218              -0.38191226
    104.773142              -0.21207061
     45.0684265             -0.02327678
     20.6137781             -0.00888124
      9.44445062            -0.00123545
      4.25252005             0.01647419
      1.87261996             0.01273639
      0.74603755             0.00097445
      0.32701681             0.00271687
      0.13158082             0.00087903
      0.05263232             0.00001929
S   20   1.00
17028964.9                   0.00004548
2186438.81                   0.00014956
 426256.871                  0.00044078
 105103.670                  0.00119126
  30487.8213                 0.00314537
   9970.05197                0.00835243
   3574.64352                0.02228196
   1376.85529                0.05706946
    560.732930               0.12885314
    238.734218               0.21986756
    104.773142               0.16046707
     45.0684265             -0.33903751
     20.6137781             -0.73165902
      9.44445062            -0.24895810
      4.25252005             0.12187451
      1.87261996             0.09637941
      0.74603755             0.00563125
      0.32701681             0.00536645
      0.13158082             0.00130610
      0.05263232            -0.00000191
S   20   1.00
17028964.9                   0.00000954
2186438.81                   0.00003137
 426256.871                  0.00009242
 105103.670                  0.00024959
  30487.8213                 0.00065822
   9970.05197                0.00174335
   3574.64352                0.00462857
   1376.85529                0.01174142
    560.732930               0.02608249
    238.734218               0.04388731
    104.773142               0.03367423
     45.0684265             -0.08460344
     20.6137781             -0.30159887
      9.44445062            -0.08554918
      4.25252005             0.52088267
      1.87261996             0.31321488
      0.74603755             0.10419005
      0.32701681             0.30149234
      0.13158082             0.12278542
      0.05263232             0.00343490
S   20   1.00
17028964.9                   0.00003652
2186438.81                   0.00012210
 426256.871                  0.00034475
 105103.670                  0.00102042
  30487.8213                 0.00222688
   9970.05197                0.00799843
   3574.64352                0.01274408
   1376.85529                0.06270798
    560.732930               0.04331676
    238.734218               0.34218226
    104.773142              -0.37655523
     45.0684265              0.60135039
     20.6137781             -4.58527400
      9.44445062             9.83946386
      4.25252005           -10.82273623
      1.87261996             7.87193392
      0.74603755            -4.96486655
      0.32701681             3.03215372
      0.13158082            -1.40779331
      0.05263232             0.43221197
S   20   1.00
17028964.9                  -0.00000974
2186438.81                  -0.00003202
 426256.871                 -0.00009439
 105103.670                 -0.00025512
  30487.8213                -0.00067393
   9970.05197               -0.00179043
   3574.64352               -0.00478391
   1376.85529               -0.01229336
    560.732930              -0.02803377
    238.734218              -0.04919004
    104.773142              -0.03856052
     45.0684265              0.10196395
     20.6137781              0.33658716
      9.44445062             0.09982437
      4.25252005            -0.58623957
      1.87261996            -0.65202065
      0.74603755             0.19039721
      0.32701681             0.67644075
      0.13158082             0.28834682
      0.05263232             0.00773775
S   20   1.00
17028964.9                   0.00000496
2186438.81                   0.00001633
 426256.871                  0.00004808
 105103.670                  0.00013052
  30487.8213                 0.00034283
   9970.05197                0.00092438
   3574.64352                0.00243820
   1376.85529                0.00649653
    560.732930               0.01461225
    238.734218               0.02788060
    104.773142               0.01897154
     45.0684265             -0.05192456
     20.6137781             -0.19758154
      9.44445062            -0.01183927
      4.25252005             0.26212428
      1.87261996             0.77019003
      0.74603755            -1.07504952
      0.32701681            -0.95261471
      0.13158082             1.28544384
      0.05263232             0.28358777
S   20   1.00
17028964.9                  -0.00001474
2186438.81                  -0.00004811
 426256.871                 -0.00014442
 105103.670                 -0.00037491
  30487.8213                -0.00107057
   9970.05197               -0.00248406
   3574.64352               -0.00810605
   1376.85529               -0.01568221
    560.732930              -0.05246215
    238.734218              -0.04879568
    104.773142              -0.12980229
     45.0684265              0.40806672
     20.6137781              0.10275696
      9.44445062             1.01672101
      4.25252005            -5.11544776
      1.87261996             8.15468363
      0.74603755            -8.77353435
      0.32701681             7.41016830
      0.13158082            -4.46801388
      0.05263232             1.64987837
S   20   1.00
17028964.9                  -0.00000837
2186438.81                  -0.00002751
 426256.871                 -0.00008120
 105103.670                 -0.00021864
  30487.8213                -0.00058110
   9970.05197               -0.00152533
   3574.64352               -0.00413567
   1376.85529               -0.01034850
    560.732930              -0.02417487
    238.734218              -0.04005295
    104.773142              -0.03521946
     45.0684265              0.09789135
     20.6137781              0.28969314
      9.44445062             0.09259601
      4.25252005            -0.79550856
      1.87261996            -0.92446399
      0.74603755             3.98830684
      0.32701681            -3.70064241
      0.13158082             0.56735426
      0.05263232             0.78318266
S   20   1.00
17028964.9                   0.00000836
2186438.81                   0.00002726
 426256.871                  0.00008226
 105103.670                  0.00021127
  30487.8213                 0.00061696
   9970.05197                0.00138151
   3574.64352                0.00477333
   1376.85529                0.00862478
    560.732930               0.03219269
    238.734218               0.02574020
    104.773142               0.08975314
     45.0684265             -0.26020098
     20.6137781              0.02962953
      9.44445062            -0.84472860
      4.25252005             2.78800390
      1.87261996            -2.63953322
      0.74603755            -0.43541455
      0.32701681             3.57225737
      0.13158082            -4.38704349
      0.05263232             2.32714970
P   17   1.00
 161308.088                  0.00004394
  24714.5235                 0.00023115
   5979.86815                0.00111396
   1880.77245                0.00496455
    697.098673               0.01956735
    287.865210               0.06479545
    128.245954               0.16887142
     60.1299881              0.31770996
     29.2171045              0.37076038
     14.4495618              0.20277004
      6.94849207             0.03882615
      3.30702782             0.00738435
      1.55878661             0.00321435
      0.60857956            -0.00000248
      0.24319665            -0.00018498
      0.09204012            -0.00006500
      0.03681605            -0.00000129
P   17   1.00
 161308.088                 -0.00001836
  24714.5235                -0.00009668
   5979.86815               -0.00046740
   1880.77245               -0.00208978
    697.098673              -0.00832989
    287.865210              -0.02811831
    128.245954              -0.07625438
     60.1299881             -0.15068312
     29.2171045             -0.18383927
     14.4495618             -0.00170180
      6.94849207             0.36782480
      3.30702782             0.50626197
      1.55878661             0.22761366
      0.60857956             0.01550742
      0.24319665            -0.00515371
      0.09204012            -0.00103363
      0.03681605            -0.00024318
P   17   1.00
 161308.088                 -0.00002255
  24714.5235                -0.00017015
   5979.86815               -0.00035348
   1880.77245               -0.00449881
    697.098673              -0.00461291
    287.865210              -0.06707370
    128.245954              -0.02976797
     60.1299881             -0.47205356
     29.2171045              0.40220449
     14.4495618             -0.95037398
      6.94849207             3.93479570
      3.30702782            -5.97900381
      1.55878661             4.63307768
      0.60857956            -2.56094402
      0.24319665             1.48590377
      0.09204012            -0.78754777
      0.03681605             0.29998365
P   17   1.00
 161308.088                  0.00000446
  24714.5235                 0.00002341
   5979.86815                0.00011373
   1880.77245                0.00050568
    697.098673               0.00203374
    287.865210               0.00683155
    128.245954               0.01881910
     60.1299881              0.03703817
     29.2171045              0.04660472
     14.4495618             -0.00704123
      6.94849207            -0.11200916
      3.30702782            -0.18498592
      1.55878661            -0.04539816
      0.60857956             0.37397099
      0.24319665             0.54205977
      0.09204012             0.23699505
      0.03681605             0.01773657
P   17   1.00
 161308.088                 -0.00000456
  24714.5235                -0.00002392
   5979.86815               -0.00011632
   1880.77245               -0.00051672
    697.098673              -0.00208072
    287.865210              -0.00698218
    128.245954              -0.01927967
     60.1299881             -0.03785375
     29.2171045             -0.04787432
     14.4495618              0.00780427
      6.94849207             0.12068833
      3.30702782             0.19099826
      1.55878661             0.07385798
      0.60857956            -0.78268398
      0.24319665            -0.16710504
      0.09204012             0.80861003
      0.03681605             0.25759175
P   17   1.00
 161308.088                  0.00001184
  24714.5235                 0.00005872
   5979.86815                0.00031868
   1880.77245                0.00121412
    697.098673               0.00587763
    287.865210               0.01618394
    128.245954               0.05718259
     60.1299881              0.08158649
     29.2171045              0.16711345
     14.4495618             -0.18553570
      6.94849207            -0.18497111
      3.30702782            -1.16000609
      1.55878661             3.04278104
      0.60857956            -3.55031625
      0.24319665             3.20774727
      0.09204012            -2.38495992
      0.03681605             1.14546896
P   17   1.00
 161308.088                  0.00000622
  24714.5235                 0.00003102
   5979.86815                0.00016602
   1880.77245                0.00064436
    697.098673               0.00303638
    287.865210               0.00854977
    128.245954               0.02892985
     60.1299881              0.04308343
     29.2171045              0.08553492
     14.4495618             -0.05748613
      6.94849207            -0.08723805
      3.30702782            -0.44589826
      1.55878661             0.22407513
      0.60857956             1.37216394
      0.24319665            -1.67772546
      0.09204012             0.22143959
      0.03681605             0.70511841
P   17   1.00
 161308.088                 -0.00000866
  24714.5235                -0.00003851
   5979.86815               -0.00025221
   1880.77245               -0.00072249
    697.098673              -0.00479644
    287.865210              -0.00910926
    128.245954              -0.04784353
     60.1299881             -0.03572518
     29.2171045             -0.17573994
     14.4495618              0.22569883
      6.94849207            -0.12994236
      3.30702782             1.23969912
      1.55878661            -1.93879496
      0.60857956             0.66010135
      0.24319665             1.05813790
      0.09204012            -2.01865715
      0.03681605             1.40553255
D   11   1.00
    560.732930               0.00068865
    238.734218               0.00240467
    104.773142               0.01433129
     45.0684265              0.05438352
     20.6137781              0.15304298
      9.44445062             0.30550848
      4.25252005             0.38567672
      1.87261996             0.29219340
      0.74603755             0.08714805
      0.29841502            -0.00020028
      0.11936601             0.00134169
D   11   1.00
    560.732930              -0.00355242
    238.734218               0.02039093
    104.773142              -0.05178080
     45.0684265              0.22138555
     20.6137781             -0.33936634
      9.44445062             2.09520411
      4.25252005            -3.07852134
      1.87261996             2.04709473
      0.74603755            -1.01273270
      0.29841502             0.50604736
      0.11936601            -0.18265878
D   11   1.00
    560.732930               0.00151526
    238.734218              -0.00473504
    104.773142               0.02283013
     45.0684265             -0.03494286
     20.6137781              0.21145080
      9.44445062            -0.13003377
      4.25252005             1.26690250
      1.87261996            -2.56827956
      0.74603755             2.33992505
      0.29841502            -1.56826608
      0.11936601             0.69379834
D   11   1.00
    560.732930              -0.00019069
    238.734218              -0.00072866
    104.773142              -0.00402111
     45.0684265             -0.01604723
     20.6137781             -0.04356888
      9.44445062            -0.09341332
      4.25252005            -0.10869852
      1.87261996            -0.09679023
      0.74603755             0.37268129
      0.29841502             0.62422320
      0.11936601             0.15811311
D   11   1.00
    560.732930               0.00023435
    238.734218               0.00066522
    104.773142               0.00471564
     45.0684265              0.01608428
     20.6137781              0.04999276
      9.44445062             0.10215584
      4.25252005             0.14963391
      1.87261996             0.14147927
      0.74603755            -1.06541591
      0.29841502             0.35047390
      0.11936601             0.68066714
D   11   1.00
    560.732930              -0.00061670
    238.734218               0.00117643
    104.773142              -0.01002897
     45.0684265              0.00264092
     20.6137781             -0.09423083
      9.44445062             0.00182149
      4.25252005            -0.45628375
      1.87261996             0.44552409
      0.74603755             0.86804683
      0.29841502            -1.76389944
      0.11936601             1.28810784
F   4   1.00
      1.417310               0.09298547
      0.566924               0.68169570
      0.226769               0.34586395
      0.090707               0.02206141
F   4   1.00
      1.417310              -0.33695994
      0.566924              -0.69024865
      0.226769               1.03430998
      0.090707               0.07354479
F   4   1.00
      1.417310               1.10050397
      0.566924              -0.97941384
      0.226769               0.08367240
      0.090707               0.60777241
F   4   1.00
      1.417310              -0.80726497
      0.566924               1.31083202
      0.226769              -1.55635355
      0.090707               1.26872782
G   2   1.00
      0.708655               0.72645609
      0.283462               0.38743584
G   2   1.00
      0.708655              -0.97944752
      0.283462               1.15626527
$end

I obtain this error after the SCF calculation ends:

SCF energy = -2605.40916475
Total energy = -2605.40916475
Q-Chem fatal error occurred in module 0, line 108:
Newton-Raphson did not converge in ShlRad

Do you know what is happening here? Thank you very much in advance for your help.

On the one hand, this crash is in a post-SCF processing step and does not affect the converged SCF energy.

Furthermore, it can be eliminated by tightening the thresholds. Using Q-Chem v. 6.2.2, the following was sufficient to eliminate this crash:

s2thresh 14
thresh 12

I have not done any further exploration, as those are my normal “tight” settings.